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[26] Li (2013) - High mobility diketopyrrolopyrrole (DPP)-based organic semiconductor materials for organic thin film transistors and photovoltaics

Come è scritta nella tesi

Li, Y., Sonar, P., Murphy, L. & Hong, W. High mobility diketopyrrolopyrrole (DPP)-based organic semiconductor materials for organic thin film transistors and photovoltaics. Energy Environ. Sci. 6, 1684 (2013).

Scheda bibliografica

Citazione completa: Li, Y.; Sonar, P.; Murphy, L.; Hong, W. High mobility diketopyrrolopyrrole (DPP)-based organic semiconductor materials for organic thin film transistors and photovoltaics. Energy & Environmental Science 2013, 6 (6), 1684. https://doi.org/10.1039/c3ee00015j

Pubblicato in: Energy & Environmental Science, vol. 6, n. 6, pp. 1684 (2013)
Editore: Royal Society of Chemistry (RSC) · tipo: journal-article
ISSN: 1754-5692, 1754-5706
Data di pubblicazione: 2013-01-01
Lingua: en

Autori e affiliazioni

Yuning Li (ORCID) - University of Waterloo
Prashant Murlidhar Sonar (ORCID) - Agency for Science, Technology and Research; Institute of Materials Research and Engineering
Leanne Murphy (ORCID) - University of Waterloo
Wei Liang Hong (ORCID) - University of Waterloo

Stato della verifica

Verificata (Crossref/OpenAlex) - fonte dati: Crossref + OpenAlex

Dove trovarla

DOI: https://doi.org/10.1039/c3ee00015j
OpenAlex: https://openalex.org/W2082306860
Accesso: closed - il testo completo richiede un abbonamento dell'editore o l'acquisto

Abstract

In recent years, the electron-accepting diketopyrrolopyrrole (DPP) moiety has been receiving considerable attention for constructing donor–acceptor (D–A) type organic semiconductors for a variety of applications, particularly for organic thin film transistors (OTFTs) and organic photovoltaics (OPVs). Through association of the DPP unit with appropriate electron donating building blocks, the resulting D–A molecules interact strongly in the solid state through intermolecular D–A and π–π interactions, leading to highly ordered structures at the molecular and microscopic levels. The closely packed molecules and crystalline domains are beneficial for intermolecular and interdomain (or intergranular) charge transport. Furthermore, the energy levels can be readily adjusted, affording p-type, n-type, or ambipolar organic semiconductors with highly efficient charge transport properties in OTFTs. In the past few years, a number of DPP-based small molecular and polymeric semiconductors have been reported to show mobility close to or greater than 1 cm2 V−1 s−1. DPP-based polymer semiconductors have achieved record high mobility values for p-type (hole mobility: 10.5 cm2 V−1 s−1), n-type (electron mobility: 3 cm2 V−1 s−1), and ambipolar (hole/electron mobilities: 1.18/1.86 cm2 V−1 s−1) OTFTs among the known polymer semiconductors. Many DPP-based organic semiconductors have favourable energy levels and band gaps along with high hole mobility, which enable them as promising donor materials for OPVs. Power conversion efficiencies (PCE) of up to 6.05% were achieved for OPVs using DPP-based polymers, demonstrating their potential usefulness for the organic solar cell technology. This article provides an overview of the recent exciting progress made in DPP-containing polymers and small molecules that have shown high charge carrier mobility, around 0.1 cm2 V−1 s−1 or greater. It focuses on the structural design, optoelectronic properties, molecular organization, morphology, as well as performances in OTFTs and OPVs of these high mobility DPP-based materials.

(Fonte: OpenAlex. Non è il testo integrale dell'articolo.)

Argomenti e parole chiave

Argomenti (OpenAlex): Organic Electronics and Photovoltaics (Electrical and Electronic Engineering); Organic Light-Emitting Diodes Research (Electrical and Electronic Engineering); Conducting polymers and applications (Polymers and Plastics)
Parole chiave: diketopyrrolopyrrole, organic thin-film transistors, organic solar cells, donor-acceptor polymers, carrier mobility, ambipolar transport, π-π stacking, energy level tuning, hole mobility, electron mobility
Concetti: Ambipolar diffusion, Organic semiconductor, Materials science, Organic solar cell, Electron mobility, Semiconductor, Acceptor, Charge carrier, Thin-film transistor, Intermolecular force

Contenuto in sintesi

Il testo completo non è ad accesso aperto e non è stato consultato: sono disponibili solo i metadati e l'abstract riportati sopra. Per approfondire, aprire la fonte dal DOI (o tramite biblioteca/abbonamento).

Come è citata nella tesi

Sez. 1.1.2 Struttura e reattività (tesi.md r. 327): Questa struttura generalmente garantisce buone proprietà conduttive, in particolare alta mobilità di carica e banda proibita a bassa energia, e consente l'applicazione del materiale in dispositivi semiconduttori come OFET e fotovoltaici organici (OPV).[25,26]

Bibliografia della fonte

La fonte cita 90 riferimenti (mostrati i primi 40; elenco completo: https://api.crossref.org/works/10.1039/c3ee00015j):

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Metriche

Citata 712 volte (OpenAlex); riferimenti nella fonte: 96
Citazioni per anno: 2026: 26, 2025: 28, 2024: 40, 2023: 34, 2022: 33, 2021: 47

Torna alla bibliografia della tesi · Generata dal catalogo bibliografia.json e da Crossref, OpenAlex, Europe PMC.

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